Engineering multilayer chemical networks

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dc.citation.titleChemical Science
dc.citation.volume10
dc.contributor.orcidhttps://orcid.org/0000-0001-6136-0980
dc.creatorMartínez-Amezaga, Maitena
dc.creatorOrrillo, Gastón
dc.creatorFurlán, Ricardo Luis Eugenio
dc.date.accessioned2024-04-15T15:16:43Z
dc.date.available2024-04-15T15:16:43Z
dc.date.issued2019
dc.description.abstractDynamic multilevel systems emerged in the last few years as new platforms to study thermodynamic systems. In this work, unprecedented fully communicated three-level systems are studied. First, different conditions were screened to selectively activate thiol/dithioacetal, thiol/thioester, and thiol/disulfide exchanges, individually or in pairs. Some of those conditions were applied, sequentially, to build multilayer dynamic systems wherein information, in the form of relative amounts of building blocks, can be directionally transmitted between different exchange pools. As far as we know, this is the first report of one synthetic dynamic chemical system where relationships between layers can be changed through network operations
dc.description.filFil: Martínez-Amezaga, Maitena. Universidad Nacional de Rosario. Facultad de Ciencias Bioquímicas y Farmacéuticas. Farmacognosia; Argentina.
dc.description.filFil: Orrillo, Gastón. Universidad Nacional de Rosario. Facultad de Ciencias Bioquímicas y Farmacéuticas. Farmacognosia; Argentina.
dc.description.filFil: Furlán, Ricardo Luis Eugenio. Universidad Nacional de Rosario. Facultad de Ciencias Bioquímicas y Farmacéuticas. Farmacognosia; Argentina.
dc.description.sponsorshipFondo para la Investigación Científica y Tecnológica (FONCYT): PICT2015-3574
dc.description.sponsorshipConsejo Nacional de Investigaciones Científicas y Técnicas (CONICET)
dc.description.sponsorshipUniversidad Nacional de Rosario (UNR)
dc.identifier.issn2041-6539
dc.identifier.urihttps://hdl.handle.net/2133/26882
dc.language.isoen
dc.publisherRoyal Society of Chemistry
dc.relation.publisherversionhttps://doi.org/10.1039/c9sc02166c
dc.relation.publisherversionhttps://pubs.rsc.org/en/content/articlepdf/2019/sc/c9sc02166c
dc.rightsopenAccess
dc.rights.holderMartínez-Amezaga, Maitena
dc.rights.holderOrrillo, Gastón
dc.rights.holderFurlán, Ricardo Luis Eugenio
dc.rights.holderUniversidad Nacional de Rosario. Facultad de Ciencias Bioquímicas y Farmacéuticas
dc.rights.textAttribution-NonCommercial 4.0 Internationalen
dc.rights.urihttp://creativecommons.org/licenses/by-nc/4.0/
dc.subjectDynamic multilevel systems
dc.subjectReversible reactions
dc.subjectDouble-level systems
dc.titleEngineering multilayer chemical networks
dc.typearticulo
dc.type.collectionarticulo
dc.type.versionpublishedVersion

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(FBIOyF) Departamento de Química Orgánica - Artículos